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RAS Chemistry & Material ScienceХимическая физика Advances in Chemical Physics

  • ISSN (Print) 0207-401X
  • ISSN (Online) 3034-6126

SOLID PRODUCTS OF NO UPTAKE ON A METHANE FLAME SOOT

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PII
S3034612625100095-1
DOI
10.7868/S3034612625100095
Publication type
Article
Status
Published
Authors
I.V. Sulimenkov
  • Affiliation: Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences
V.V. Filatov
  • Affiliation: Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences
V.S. Brusov
  • Affiliation: Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences
E.V. Aparina
  • Affiliation: Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences
V. V. Zelenov
  • Affiliation: Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences
Volume/ Edition
Volume 44 / Issue number 10
Pages
93-102
Abstract
Modern global models used for long-term prediction of the chemical composition of the Earth’s atmosphere require detailed information on the rate constants of numerous elementary chemical reactions. In addition, data on the composition of the reaction products is also of great importance. In this work, high-resolution mass spectrometry was used to identify the solid products of soot nitration by dinitrogen pentoxide (NO) during methane combustion. A high reactivity of NO toward polycyclic aromatic hydrocarbons (CH class) present in the initial soot was established. It was shown that the solid nitration products include nitro derivatives of polycyclic aromatic compounds, aromatic acids, and their esters. In terms of composition and compound classes, the products of soot nitration by NO are similar to those obtained in nitration by nitrogen dioxide (NO).
Keywords
химия тропосферы NO сажа твердые продукты реакции масс-спектрометрия
Date of publication
21.04.2025
Year of publication
2025
Number of purchasers
0
Views
38

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